To tame a higher level use starve tame.

Use a bola so it can not fly away.

Use tranqs

Best to feed dodo kibble to keep taming effectiveness higher.

Build spike walls around to protect from predators

Once tamed take to the skies just make sure you watch it's stamina as you can easily land in or around a swamp area with titanboas around to poison and kill you and your tame.

More Pteranodon Taming & KO Tips