Megalooceros are easy tame because they are passive but once hit they run away which is bad for itself and you because it will run into other creatures. Such Rexes, raptors, sarbertooths, scorpions, Argys, allosaurus, thylas, yutys, daedons, and Carnos. Also other dangerous creatures. All you need are bolas to trap it, tranq arrows or a club to knock it out, and berries or crops to feed it. And done have a good day with your deer.

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