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Knocking out a high level lymantria within a single bola is impossible with a primitive crossbow. Instead, quickslot two pillars, two thatch ceilings, and five thatch walls. Bola the moth over flat land, then drop a pillar on one side. Ceilings next over it, then the other pillar on the other side. Hang walls from the ceilings. When it comes out of the bola, it's trapped. Tranq slowly so it won't die, and leave the trap up as a tame blind during taming. If you fail to trap it just try again; it won't flee far after a bola attack if you did no other attacks.

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